From: Cynthia Twohy
Organization: Oregon State University/NCAR
Research Area: AEROSOLS
Mission Scenario: New Particle Production Near Convective Cloud Outflow
Recent studies suggest that the production of new particles may be
favored downstream of the outflow of convective cloud systems in the
upper troposphere. Cold temperatures, low particle surface area, and
high levels of gas-phase precursers carried up by the convection
provide ideal conditions for the nucleation of ultrafine sulfuric acid
particles. These will then grow by coagulation to larger particles,
which may be important for chemical reactions or cloud formation.
Although the tropical upper troposphere provides widespread convection
and cold temperature extremes, these events may occur near
mid-latitude storms as well. Measurements of new particle formation
have been sporadic, since the nucleation process requires special
conditions and the environment is difficult to sample. Also,
observations may occur inadvertently while conducting other
measurements. Existing data sets are incomplete because instruments
and flight plans have not been selected specifically for this problem.
HIAPER, with its long range, high ceiling, and large payload capacity,
should be ideal to study the problem.
Flight Plan:
Similar flights would be planned for both mid-latitude and tropical
regions on different days, so an intermediate base, perhaps in Mexico,
might be appropriate. Using forecasts and satellite imagery to target
regions of active convection, the aircraft would ferry to the
equatorial region (2.75 hrs), receiving on-board satellite updates to
refine the target area. Once there, we would sample the ambient
aerosol at high altitude and select an isolated cloud system in active
development with anvil just beginning to form (0.5 hrs). Aircraft
would descend to just above the surface at 1000 ft/min (0.75 hrs). If
possible, aircraft would then circumnavigate the storm near the
surface to measure chemistry and state parameters of the inflow
region, then ascend (1.5 hrs). The first upper level would be 1000 ft
below the cirrus outflow, at its furthest downwind end. A race track
pattern would be conducted across the cirrus band, half below the
visible cloud and half downwind. This would be repeated at the cirrus
level and 1000 ft above it (1.25 hrs). (If additional time is
available, the aircraft would loiter in the downwind region attempting
to measure particle evolution over time.) Ferry home (2.75 hrs).
Total flight time: 9.5 hrs.
Alternately, the mid-latitude portions of the experiment could be
based in Jeffco, with the aircraft moving to Panama for the tropical
missions. With more time on station in both sites, these flights
could perhaps be combined with some of the related missions of others
(Clarke, Young, Toon).
Instrumentation:
- State Parameters
- Community Aerosol Inlet
- Ultrafine CN (surface to 50Kft)
- Aerosol Particle Size Distribution, 0.01 to 1.0 micron
- Cloud (Liquid and Ice) Particle Size Distribution, 1.0 to 500 micron
- Gas-Phase Chemistry (SO2, H2SO4, OH radical, NOx)
- Aerosol Chemistry (Electron Microscope and Mass Spectrometry)
- Radiation: uv
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